So, it's gone a bit better but still needs work. The mix was perfect, so that is something, fully set already this morning:

- IMG20240725092508.jpg (220.17 KiB) Viewed 736 times
It isn't without issues though:

- IMG20240725092540.jpg (144.83 KiB) Viewed 736 times
Unfortunately the blue cube mould got an air bubble in it at the fill hole, however the finish and weight of the cast ball was pretty good, and I can try again, but now just need to be sure I have a process to avoid air bubbles.
The spherical mould worked well from a size/weight perspective, however the alignment was poor leaving a lot of flashing on the edge:

- IMG20240725092524.jpg (143.56 KiB) Viewed 736 times
For reference I weighed some of the mice ball replacements I have, plus actual balls, results below.
20mm steel ball:

- IMG_20240725_093032.jpg (277.46 KiB) Viewed 736 times
20mm delrin ball:

- IMG20240725093057.jpg (228.75 KiB) Viewed 736 times
22mm mouse ball

- IMG20240725093231.jpg (258.47 KiB) Viewed 736 times
Hand rolled 'Milliput' (Epoxy filler):

- IMG20240725093117.jpg (249.74 KiB) Viewed 736 times
20mm rubber ball:

- IMG20240725093130.jpg (225.96 KiB) Viewed 736 times
20mm resin only ball:

- IMG20240725093150.jpg (267.03 KiB) Viewed 736 times
20mm resin/iron powder composite ball from spherical mould:

- IMG20240725093204.jpg (261.12 KiB) Viewed 736 times
20mm resin/iron powder composite ball from the blue cube mould made by me:

- IMG20240725093219.jpg (233.12 KiB) Viewed 736 times
I think the other ball from the spherical mould is representative of the finished weight of the blue cube ball if it wasn't missing a piece given the air bubble it suffered.
Given the weight of the 22mm mouse ball, I think that 20mm composite ball is really quite close weight wise and far better then the other offerings, such as rubber or delrin, and the steel is rather too heavy.
I think I will give the blue cube another go, and I may also try making a new mould from the 20mm steel ball in which I can suspend a smaller steel ball and pour RTV silcone round it like a normal ball.